
Visible light leaves evaporation and interfacial structure of neat water unchanged at the air-water interface.
Visible light-induced "photomolecular" enhancement of water evaporation has been proposed as a fundamentally new mode of light-matter interaction at aqueous interfaces, with far-reaching implications for climate processes and light-driven water technologies. Yet, the response of neat interfacial water to visible photons has not been directly quantified at both macroscopic and molecular scales. Here, we combine high-precision confocal displacement measurements with a surface-specific vibrational
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